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DTSTART:20260319T100000Z
SEQUENCE:0
TRANSP:OPAQUE
LOCATION:Elements Room
SUMMARY:ICFO | SAAD ABDULLAH  
CLASS:PUBLIC
DESCRIPTION:Technological progress in the twenty first century increasingly
  relies on the ability to control light and electromagnetic fields across 
 multiple spatial and spectral scales. As device dimensions shrink\, strong
  confinement becomes essential\, and plasmons\, the collective oscillation
 s of conduction electrons in metals\, provide an efficient route to concen
 trate optical fields far below the diffraction limit and enhance light mat
 ter interactions. In this thesis\, we engineer and study strongly confined
  optical fields in nanoengineered metallic systems\, where plasmonic reson
 ances play a central role in shaping both linear response and nonlinear em
 ission.\nIn the first part\, we study scatterer assisted coupling of free 
 space radiation into surface supported plasmonic modes\, which cannot be e
 fficiently excited by direct illumination due to strong momentum mismatch.
  We show that metallic nanodisks placed near a plasmon supporting interfac
 e can launch surface plasmons\, with coupling governed by disk position an
 d distance from the surface. By tuning the nanodisk size\, we control its 
 resonance wavelength and access a wide near infrared to infrared spectral 
 region. We further investigate periodic nanodisk arrays\, where lattice re
 sonances reshape the scattering response and shift the optimal scatterer t
 o substrate distance. By tuning the array geometry\, we identify configura
 tions that maximize coupling and determine optimal launching conditions. R
 esults are supported by analytical modelling and numerical simulations.\nT
 he second part focuses on ultrathin epitaxial crystalline silver films wit
 h thicknesses of only a few tens of monolayers\, approaching the monolayer
  limit. These films provide strong intrinsic confinement and support high 
 quality resonances over a broad spectral range spanning the visible and ne
 ar infrared. We investigate patterned geometries including ribbons\, nanot
 riangles\, bow tie antennas\, and rods\, and demonstrate robust tunability
  with quality factors approaching\, and for optimal configurations reachin
 g\, values on the order of 11. We compare pre patterned and post patterned
  fabrication approaches and show that suitable capping layers suppress dew
 etting and ensure long term stability. Despite their reduced thickness\, w
 e show that their optical response can be described using a modified Drude
  model with increased damping to account for confinement and fabrication r
 elated losses.\nFinally\, we investigate the nonlinear optical response of
  these ultrathin metal systems with emphasis on second harmonic generation
 . In ultrathin crystalline films\, strong interfacial symmetry breaking an
 d vertical confinement enable a measurable nonlinear response. We show tha
 t decreasing film thickness enhances the second harmonic signal\, and that
  resonant nanopatterning\, particularly using stable capped silver nanorib
 bon arrays\, yields broad tunability and strong plasmon enhanced near fiel
 ds\, producing conversion efficiencies a few orders of magnitude higher th
 an planar films under resonant excitation.\nOverall\, this work highlights
  plasmon enabled nanoengineering as a powerful route to control and concen
 trate light beyond the diffraction limit\, enabling compact nonlinear phot
 onic architectures\, silicon compatible frequency conversion\, and emergin
 g quantum photonic technologies.\nThursday March 19\, 11:00 h. Elements Ro
 om\nThesis Director: Prof. Dr. Javier Garc&iacute\;a de Abajo and Dr. Vaha
 gn Mkhitaryan
DTSTAMP:20260417T125144Z
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